Optical and transport properties of NbN thin films revisited
arxiv(2024)
摘要
Highly disordered NbN thin films exhibit promising superconducting and
optical properties. Despite extensive study, discrepancies in its basic
electronic properties persist. Analysis of the optical conductivity of
disordered ultra-thin NbN films, obtained from spectroscopic ellipsometry by
standard Drude-Lorentz model, provides inconsistent parameters. We argue that
this discrepancy arise from neglecting the presence of quantum corrections to
conductivity in the IR range. To resolve this matter, we propose a modification
to the Drude-Lorentz model, incorporating quantum corrections. The parameters
obtained from the modified model are consistent not only with transport and
superconducting measurements but also with ab initio calculations. The
revisited values describing conduction electrons, which differ significantly
from commonly adopted ones, are the electron relaxation rate
Γ≈1.8 eV/ħ, the Fermi velocity v_F ≈ 0.7
× 10^6 ms^-1 and the electron density of states
N(E_F)=2states of both spins/eV/V_f.u..
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