Gamma-ray Spectroscopy in Low-Power Nuclear Research Reactors

Oskari V. Pakari, Andrew Lucas,Flynn B. Darby,Vincent P. Lamirand,Tessa Maurer, Matthew G. Bisbee, Lei R. Cao,Andreas Pautz,Sara A. Pozzi

JOURNAL OF NUCLEAR ENGINEERING(2024)

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摘要
Gamma-ray spectroscopy is an effective technique for radioactive material characterization, routine inventory verification, nuclear safeguards, health physics, and source search scenarios. Gamma-ray spectrometers typically cannot be operated in the immediate vicinity of nuclear reactors due to their high flux fields and their resulting inability to resolve individual pulses. Low-power reactor facilities offer the possibility to study reactor gamma-ray fields, a domain of experiments hitherto poorly explored. In this work, we present gamma-ray spectroscopy experiments performed with various detectors in two reactors: The EPFL zero-power research reactor CROCUS, and the neutron beam facility at the Ohio State University Research Reactor (OSURR). We employed inorganic scintillators (CeBr3), organic scintillators (trans-stilbene and organic glass), and high-purity germanium semiconductors (HPGe) to cover a range of typical-and new-instruments used in gamma-ray spectroscopy. The aim of this study is to provide a guideline for reactor users regarding detector performance, observed responses, and therefore available information in the reactor photon fields up to 2 MeV. The results indicate several future prospects, such as the online (at criticality) monitoring of fission products (like Xe, I, and La), dual-particle sensitive experiments, and code validation opportunities.
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关键词
gamma-ray spectroscopy,research reactors,fission products,CeBr3,high-purity germanium,stilbene,organic glass
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