Disordered ground state in the spin-orbit coupled Jeff=1/2 distorted honeycomb magnet BiYbGeO5

S. Mohanty, S. S. Islam, N. Winterhalter-Stocker, A. Jesche, G. Simutis,Ch Wang, Z. Guguchia, J. Sichelschmidt, M. Baenitz, A. A. Tsirlin, P. Gegenwart,R. Nath

PHYSICAL REVIEW B(2023)

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摘要
We delineate quantum magnetism in the strongly spin-orbit coupled distorted honeycomb lattice antiferromagnet BiYbGeO5. Our magnetization and heat capacity measurements reveal that its low-temperature behavior is well described by an effective J(eff) = 1/2 Kramers doublet of Yb3+. The ground state is nonmagnetic with a tiny spin gap. Temperature-dependent magnetic susceptibility, magnetization isotherm, and heat capacity can be modeled well assuming isolated spin dimers with anisotropic exchange interactions J(Z) similar or equal to 2.6 K and J(XY) similar or equal to 1.3 K. Heat capacity measurements backed by muon spin relaxation suggest the absence of magnetic long-range order down to at least 80 mK both in zero field and in applied fields. This sets BiYbGeO5 apart from Yb2Si2O7, with its unusual regime of magnon Bose-Einstein condensation, and suggests negligible interdimer couplings, despite only a weak structural deformation of the honeycomb lattice.
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