Interface-suppressed high-quality symmetrical bifacial flexible CZTSe solar cells through a green electrodeposition process
JOURNAL OF MATERIALS CHEMISTRY A(2023)
摘要
Bifacial flexible solar cells are considerably attractive owing to their high generation of energy per area and multidirectional light irradiation in advanced applications, such as building-integrated photovoltaics. Their technological ability to reduce manufacturing costs and time is highly essential. Although the solution-processed technique has implemented bifacial flexible Cu2ZnSn(S,Se)4 (CZTSSe) solar cells, no progress on the green electrodeposition process has occurred. Herein, we first propose symmetrical bifacial Cu2ZnSnSe4 (CZTSe) solar cells through a facile electrodeposition process, in which Mo foils are used as a common back electrode for both sides. Stacked electrodeposition accomplished at one time is involved to produce high-quality bifacial CZTSe absorber layers. This strategy can guarantee the consistency of bifacial flexible solar cells and immensely low costs and time. The resultant high efficiencies of 6.43% and 6.20% for the two sides have made a great breakthrough for electrodeposited flexible CZTSSe devices and offered a cost-effective strategy for green-processed material fabrications. Compared with the solution-processed technique, the determined interfacial-suppressed Voc limiting the efficiency provides a clear aspect for further improving the efficiency. A symmetrical bifacial flexible Cu2ZnSnSe4 (CZTSe) solar cells are fabricated through a green electrodeposition process with championed efficiencies for both sides.
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关键词
solar cells,high-quality
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