Laser cooling of positronium

When laser radiation is skilfully applied, atoms and molecules can be cooled allowing precise measurements and control of quantum systems. These are essential in fundamental studies of physics as well as practical applications such as precision spectroscopy, quantum-statistical-property manifesting ultracold gases, and quantum computing. In laser cooling, repeated cycles of laser photon absorption and direction-independent spontaneous emission can slow atoms and molecules to otherwise unattainable velocities. Simple systems can provide a rigorous testing ground for fundamental theories of physics; one such system is the purely leptonic positronium, an exotic atom of an electron and its antiparticle, the positron. However, the cooling of positronium has hitherto remained unrealised. Here, we demonstrate laser cooling of positronium. A novel laser system of a train of broadband pulses with successively increasing central frequencies was used to overcome major challenges presented by the short lifetime of positronium and the significant Doppler broadening and recoil as a consequence of its very light mass. One-dimensional chirp cooling of the dilute positronium gas in a counter-propagating configuration gave a final velocity distribution corresponding to approximately 1 K in a short time of 100 ns. This study on a pure leptonic system is a major step in the field of low-temperature fundamental physics of antimatter, and is complementary to the laser cooling of antihydrogen, a hadron-containing atom. Progress in this field is vital in elucidating the origin of the matter-antimatter asymmetry in the universe. The application of laser cooling to positronium may afford a unique opportunity to rigorously test bound-state quantum electrodynamics. Moreover, laser cooling of positronium is key to the realisation of Bose-Einstein condensation in this matter-antimatter system.