Mechanically Tough and Highly Stretchable Hydrogels Based on Polyurethane for Sensitive Strain Sensor.
Polymers(2023)
摘要
Hydrogels with flexible and stretchable properties are ideal for applications in wearable sensors. However, traditional hydrogel-based sensors suffer from high brittleness and low electrical sensitivity. In this case, to solve this dilemma, a macromolecular polyurethane crosslinking agent (PCA) was designed and prepared; after that, PCA and two-dimensional (2D) MXene nanosheets were both introduced into a covalently crosslinked network to enhance the comprehensive mechanical and electrochemical properties of the hydrogels. The macromolecular polyurethane crosslinking agent promotes high-tensile strength and highly stretchable capacity by suitable covalent crosslinking. The optimized hydrogel, which exhibited maximum tensile strength and maximum elongation at break, had results of 1.21 MPa and 644%, respectively. Two-dimensional MXene nanosheets provide hydrogel with high electrical conductivity and strain sensitivity, producing a wearable device for the continuous monitoring of human movements and facial microexpressions. This study demonstrated an efficient structure design strategy for building mechanically tough, highly stretchable, and sensitive dual-mode MXenes-based wearable sensors.
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关键词
stretchable hydrogels,polyurethane,strain
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