Imaging the suppression of ferromagnetism in LaMnO_3 by metallic overlayers
arxiv(2023)
摘要
LaMnO_3 (LMO) thin films epitaxially grown on SrTiO_3 (STO) usually
exhibit ferromagnetism above a critical layer thickness. We report the use of
scanning SQUID microscopy (SSM) to study the suppression of the ferromagnetism
in STO/LMO/metal structures. By partially covering the LMO surface with a
metallic layer, both covered and uncovered LMO regions can be studied
simultaneously. While Au does not significantly influence the ferromagnetic
order of the underlying LMO film, a thin Ti layer induces a strong suppression
of the ferromagnetism, over tens of nanometers, which increases with time on a
timescale of days. Detailed EELS analysis of the Ti-LaMnO_3 interface reveals
the presence of Mn^2+ and an evolution of the Ti valence
state from Ti^0 to Ti^4+ over approximately 5 nanometers. Furthermore, we
demonstrate that by patterning Ti/Au overlayers, we can locally suppress the
ferromagnetism and define ferromagnetic structures down to sub-micrometer
scales.
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