Insights into quantitative evaluation technology of PM2.5 transport at multi-perspective and multi-spatial and temporal scales in the north China plain

Cross-border transport is a crucial factor affecting air quality, while how to quantify the transport contribution through different technologies at multi-perspective and multi-scale have not been fully understood. This study established three quantification techniques, and conducted a systematic assessment of PM2.5 transport over the North China Plain (NCP) based on numerical simulations and vertical observations. Results suggested that the annual local emissions, inter-urban and outer-regional transport contributed 44.5%-64.6%, 15.2%-27.9% and 18.0%-28.2% of total surface PM2.5 concentrations, respectively, with transport intensity stronger in July and April, yet weaker in January and October. The southwest-northeast, northeast-southwest, and south-east-northwest were three prevailing transport directions near the surface. By comparison, the annual PM2.5 transport contribution below the atmospheric boundary layer height increased by 16.8%-24.5% in Beijing, Tianjin and Shijiazhuang, with inter-urban and outer-regional contribution of 29.8%-32.1% and 18.5%-23.1%. Furthermore, observed fluxes from fixed-point and vehicle-based mobile lidar were in good agreement with the simulated flux. PM2.5 net flux intensity varied with height, with generally larger at the middle-and high-altitude layer than that of low-altitude layer. In the early, during and late period of haze peak formation (Stage I, II, III, respectively), the largest absolute flux intensity on average was Stage II (566.7 t/d), followed by Stage III (307.0 t/d) and I (191.4 t/d). Besides, external transport may dominate the second concentration peak, while local emissions may play a more vital role in the first and third peaks. It has been noted that joint prevention and control measures should be proposed 1-2 days before reaching PM2.5 extremes. These findings could improve our understanding of transport influence mechanism of PM2.5 and propose effective emission reduction measures in the NCP region.