Giant nonlinear Hall effect in twisted bilayer WSe2

Abstract The recently discovered nonlinear Hall effect (NHE) in a few non-interacting systems provides a novel mechanism for generating second harmonic electrical Hall signals under time-reversal-symmetric conditions. Here, we introduce a new approach to engineering NHE by using twisted moiré structures. We found that the twisted WSe2 bilayer exhibited a NHE when the Fermi level was tuned to the moiré flat bands. When the first moiré band was half-filled, the nonlinear Hall signal exhibited a sharp peak with a generation efficiency that was at least two orders of magnitude greater than those obtained in previous experiments. We discuss the possible origins of the diverging generation efficiency in twisted WSe2 based on resistivity measurements, such as moiré interface induced correlation effects and mass-diverging type continuous Mott transition. This study demonstrates not only how interaction effects can combine with Berry curvature dipoles to produce novel quantum phenomena, but also the potential of NHE measurements as a new tool for studying quantum criticality.