THz Ultra-Strong Light-Matter Coupling up to 200 K with Continuously-Graded Parabolic Quantum Wells

ADVANCED OPTICAL MATERIALS(2023)

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摘要
Continuously graded parabolic quantum wells with excellent optical performances are used to overcome the low-frequency and thermal limitations of square quantum wells at terahertz (THz) frequencies. The formation of microcavity intersubband polaritons at frequencies as low as 1.8 THz is demonstrated, with a sustained ultra-strong coupling regime up to a temperature of 200 K. Thanks to the excellent intersubband transition linewidth, polaritons present quality factors up to 17. It is additionally shown that the ultra-strong coupling regime is preserved when the active region is embedded in sub-wavelength resonators, with an estimated relative strength eta = omega(R)/omega(0) = 0.12. This represents an important milestone for future studies of quantum vacuum radiation because such resonators can be optically modulated at ultrafast rates, possibly leading to the generation of non-classical light via the dynamic Casimir effect. Finally, with an effective volume of 2x10-6 lambda 03$2{\bm{ \times }}{10<^>{{\bm{ - }}6}}\lambda _0<^>3$, it is estimated that fewer than 3000 electrons per resonator are ultra-strongly coupled to the quantized electromagnetic mode, proving it is also a promising approach to explore few-electron polaritonic systems operating at relatively high temperatures.
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关键词
intersubband,metamaterials,polaritons,terahertz
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