Unraveling Dipolar Regime and Kerker Conditions in Mid-Index Mesoscale Dielectric Materials

ADVANCED OPTICAL MATERIALS(2023)

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摘要
Nanophotonic phenomena, such as zero optical back scattering, nonradiating anapole states, etc. are related to the excitation of single dipolar modes-hence so far, they have only been observed within a few relatively high-index dielectric materials (refractive index, n > 3.5) in the nanoscale regime at the optical frequencies. Here, dipolar regime is unraveled, close-to-zero backscattering is demonstrated, and optical anapoles are excited in mid-index dielectric spheres (titanium di-oxide, TiO2; n approximate to 2.6) at the mesoscale regime (particle diameter, d approximate to incident wavelength, lambda) under illumination with tightly focused Gaussian beams (TFGBs). Successive scattering minima associated with dipolar excitation are observed satisfying the first Kerker condition in the scattering spectra of single TiO2 spheres with diameters in the micrometer range. Moreover, at specific wavelengths, the electric and magnetic dipolar scattering amplitudes of the dielectric microspheres simultaneously go close-to-zero, leading to the excitation of hybrid optical anapoles with a total scattering intensity approximate to 5 times weaker for TFGB illumination with numerical aperture, NA approximate to 0.95 compared to NA approximate to 0.1. The result pushes the boundary of the observation of nanophotonic phenomena to a new regime with regards to type and size of the materials.
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关键词
Kerker condition,mesoscale interactions,mid-index materials,nanophotonics,optical spectroscopy,optical anapole,zero backscattering
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