Colossal Room-Temperature Terahertz Topological Response in Type-II Weyl Semimetal NbIrTe4

Advanced Materials(2022)

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摘要
The electromagnetic spectrum between microwave and infrared light is termed the "terahertz (THz) gap," of which there is an urgent lack of feasible and efficient room-temperature (RT) THz detectors. Type-II Weyl semimetals (WSMs) have been predicted to host significant RT topological photoresponses in low-frequency regions, especially in the THz gap, well addressing the shortcomings of THz detectors. However, such devices have not been experimentally realized yet. Herein, a type-II WSM (NbIrTe4) is selected to fabricate THz detector, which exhibits a photoresponsivity of 5.7 x 10(4) V W-1 and a one-year air stability at RT. Such excellent THz-detection performance can be attributed to the topological effect of type-II WSM in which the effective mass of photogenerated electrons can be reduced by the large tilting angle of Weyl nodes to further improve mobility and photoresponsivity. Impressively, this device shows a giant intrinsic anisotropic conductance (sigma(max)/sigma(min) = 339) and THz response (Iph-max/Iph-min = 40.9), both of which are record values known. The findings open a new avenue for the realization of uncooled and highly sensitive THz detectors by exploring type-II WSM-based devices.
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关键词
anisotropy, terahertz detectors, type-II Weyl semimetals
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