Pushing the polariton confinement limits with low losses using image polaritons in boron nitride

arxiv(2020)

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摘要
Polaritons in two-dimensional (2D) materials provide extreme light confinement that is not possible with conventional metal plasmonics. However, such large confinement inevitably increases optical losses through various damping channels. Here we demonstrate that a hyperbolic phonon polariton (HPhP) mode in hexagonal boron nitride (hBN) can overcome the fundamental trade-off, featuring ultra-tight confinement and exceptional quality factors simultaneously. Compared to its charge-symmetric counterpart, the HPhP mode with anti-symmetric charge distributions exhibits lower optical losses while also acquiring tighter polariton confinement that is not limited by Landau damping due to the bosonic nature of HPhPs. Far-field observation of this high-momenta anti-symmetric mode becomes possible with our resonator design that can boost the coupling efficiency by launching a virtual polariton mode with image charges, while using hBN isotopically enriched in $^{10}$B with low optical losses. We experimentally observed a record-high effective index of up to 132 and quality factors as high as 501, values much higher than found in hBN with the natural distribution of boron isotopes. Our phenomenological theory suggests an important role of hyperbolic surface scattering in the damping process of HPhPs. Our image-polariton resonator scheme is universally applicable to polaritons in 2D materials and enable the extreme engineering of modal properties and light-matter interactions.
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关键词
polariton confinement limits,boron nitride,image polaritons
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