Coherence limit due to hyperfine interaction with nuclei in the barrier material of Si spin qubits
arxiv(2024)
摘要
On the quest to understand and reduce environmental noise in Si spin qubits,
hyperfine interactions between electron and nuclear spins impose a major
challenge. Silicon is a promising host material because one can enhance the
spin coherence time by removing spinful ^29Si isotopes. As more experiments
rely on isotopic purification of Si, the role of other spinful atoms in the
device should be clarified. This is not a straightforward task, as the
hyperfine interactions with atoms in the barrier layers are poorly understood.
We utilize density functional theory to determine the hyperfine tensors of both
Si and Ge in a crystalline epitaxial Si/SiGe quantum well as well as Si and O
atoms in an amorphous Si/SiO_2 (MOS) interface structure. Based on these
results, we estimate the dephasing time T_2^* due to magnetic noise from the
spin bath and show that the coherence is limited by interactions with non-Si
barrier atoms to a few µs in Si/SiGe (for non-purified Ge) and about
100 µs in Si-MOS. Expressing these numbers alternatively, in Si/SiGe
the interactions with Ge dominate below 1000 ppm of ^29Si content, and,
due to low natural concentration of the spinful oxygen isotopes, the
interactions with oxygen in Si-MOS become significant only below 1 ppm of
^29Si content.
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