La doping greatly enhances electrochemical alkaline seawater oxidation over Ni(OH)2 nanosheet
CATALYSIS SCIENCE & TECHNOLOGY(2024)
摘要
The utilization of seawater electrolysis is recognized as a promising method for generating H-2 as a substitute for conventional technology. Nevertheless, it is impeded by anode catalysts with restricted lifespans, primarily due to chloride-induced competitive chemical reactions. This study reports an La-doped Ni(OH)(2) nanosheet supported on Ni foam (La-Ni(OH)(2)/NF) as an outstanding oxygen evolution reaction electrocatalyst, which demonstrates remarkable performance in alkaline seawater. Impressively, the achievement of a high current density (500 mA cm(-2)) requires a low overpotential of only 434 mV, surpassing that of Ni(OH)(2)/NF (532 mV). In addition, La-Ni(OH)(2)/NF exhibits outstanding electrochemical stability for the duration of more than 200 h in alkaline seawater.
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