Progressive polymer deformation induced by polar activity and the influence of inertia
arxiv(2024)
摘要
Polar activity is shown here to induce a progressive local deformation of
linear polymer chains, making a clear distinction between head and tail, while
the overall chain conformation gets more compact. This breakdown of
self-similarity, provoked by the accumulated tension on the polymer backbone
induced by the activity, is shown to occur both in the absence and presence of
inertia, although it is stronger in the latter case. Other properties like the
relaxation time and diffusion are also largely influenced by the presence of a
polar activity.
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