Measurement of the neutron capture cross sections of rhenium up to stellar s- and r-process temperatures at the China Spallation Neutron Source Back-n facility

PHYSICAL REVIEW RESEARCH(2024)

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摘要
The neutron capture measurement of natural rhenium was performed with the time -of -flight technique at the Back -n facility of the China Spallation Neutron Source in the energy range from 1 to 500 eV of the resolved resonance region (RRR) and from 5 to 400 keV in the unresolved resonance region (URR). Prompt gamma-rays originating from neutron -induced capture events were detected by four C6D6 detectors. The pulse height weighting technique and the double -bunch unfolding method based on the Bayesian theory were used in the data analysis. To obtain reliable measurement results, background subtraction, normalization, and corrections were carefully considered. The multilevel R -matrix Bayesian code SAMMY was used to extract the resonance parameters in the RRR. An absence of resonance near 392 eV is observed in our measurement, which has been observed in previous works. The average cross sections in the URR of natural rhenium relative to 197Au were obtained in logarithmical equidistant energy bins with 20 bins per energy decade. The TALYS code was used to describe the average cross sections in the URR; the Maxwellian-averaged cross sections (MACSs) of 185Re and 187Re are given from kT = 5 to 100 keV. At a thermal energy of kT = 30 keV, the MACS value for 185Re (1469 +/- 127 mb) is in good agreement with the Karlsruhe Astrophysical Database of Nucleosynthesis in Stars (KADoNIS) recommended value (1535 +/- 62 mb) within the error bars. By contrast, the value of 1361 +/- 118 mb for 187Re shows a discrepancy with the KADONIS recommended value (1160 +/- 57 mb).
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