Stereodivergent Synthesis of Chiral Spiropyrazolones through Pd-Catalyzed Asymmetric Sequential Hydroalkylation of 1,3-Enynes: Unusual Solvent Effect on the Enantioselectivity

Shan Wang,Long Li, Yifei Zheng, Luqing Li,Yingcheng Wang,Fangzhi Peng,Zhihui Shao

Organic Chemistry Frontiers（2024）

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摘要

Chiral spiropyrazolones were constructed for the first time through Pd-catalyzed asymmetric sequential hydroalkylation of 1,3-enynes. Through substrate control (by exchanging the position of double bond and triple bond of 1,3-enyne...

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