Strain-induced enhancement of the charge-density-wave in the kagome metal ScV_6Sn_6
arxiv(2024)
摘要
The kagome geometry is an example of frustrated configuration in which rich
physics takes place, including the emergence of superconductivity and charge
density wave (CDW). Among the kagome metals, ScV_6Sn_6 hosts an
unconventional CDW, with its electronic order showing a different periodicity
than that of the phonon which generates it. In this material, a CDW-softened
flat phonon band has a second-order collapse at the same time that the first
order transition occurs. This phonon band originates from the out-of-plane
vibrations of the Sc and Sn atoms, and it is at the base of the
electron-phonon-coupling driven CDW phase of ScV_6Sn_6. Here, we use
uniaxial strain to tune the frequency of the flat phonon band, tracking the
strain evolution via time-resolved optical spectroscopy and first-principles
calculations. Our findings emphasize the capability to induce an enhancement of
the unconventional CDW properties in ScV_6Sn_6 kagome metal through control
of strain.
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