Breaking the Sabatier’s Vertex via Switching the Oxygen Adsorption Configuration and Reaction Pathway on Dual-active Sites for Acidic Oxygen Reduction

Pan Guo,Bo Liu,Fengdi Tu,Yunkun Dai,Ziyu Zhang,Yunfei Xia,Miao Ma,Yunlong Zhang,Lei Zhao,Zhenbo Wang

Energy & Environmental Science（2024）

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摘要

The single-atom catalysts are promising alternatives to platinum-based catalysts for oxygen reduction reaction (ORR). However, the ORR process with multiple-step proton-coupled electron transfer occurring on the single-active site follows the...

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