Liquid-liquid flow pattern and mass transfer in a rotating millimeter channel reactor

CHEMICAL PRODUCT AND PROCESS MODELING(2024)

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摘要
Currently, microchannels are widely used in liquid-liquid heterogeneous mass transfer systems due to its excellent mass transfer performance. However, because of the passive mixing principle of traditional microchannels, the improvement of mass transfer performance has a bottleneck. This work proposes a novel rotating millimeter channel reactor (RMCR), capable of achieving liquid-liquid heterogeneous mass transfer enhance by centrifugal force. Three typical flow patterns of slug flow, parallel-droplet flow, and parallel flow in the RMCR were observed by high-speed photography technology. The volumetric mass transfer coefficient (K O a) of the RMCR increased with the increase of the total volumetric flow rate and rotational speed (N) increased. Compared with N = 0 r/min, the K O a of the RMCR increases by 61.5 % at 200 r/min, ranging from 0.013 to 0.021 s(-1). The RMCR proposed in this work is expected to be applied to the liquid-liquid heterogeneous mass transfer system with high processing capacity and easy plugging.
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关键词
rotating millimeter channel reactor,liquid-liquid heterogeneous,flow pattern,mass transfer
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