Mg(II)-Catalyzed [4+2] Annulation for the Synthesis of 2-Arylquinoline Motifs: Applications and DFT Studies

Tao Yang, Yibo Qin, Yaping Wang, Fu Song,Heng-Ying Xiong,Teng Wang,Guangwu Zhang

ADVANCED SYNTHESIS & CATALYSIS（2024）

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摘要

Mg-catalyzed [4+2] cycloaddition reactions between 2-aminobenzaldehydes and ynones offered an array of 2-arylquinoline motifs merged with a CF3-acyl group. Furthermore, with Mg-catalyzed [4+2] annulation as the key step, DDD107498, DDD102542, and Hit analogues were assembled. Finally, a computational study of the reaction mechanism was conducted. image

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关键词

Quinoline,[4+2] Annulation,Magnesium

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