Chirped amplitude mode in photo-excited superconductors

Thomas Blommel,Jason Kaye,Yuta Murakami, Emanuel Gull,Denis Golež

arxiv(2024)

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摘要
We show that the amplitude mode in superconductors exhibits chirped oscillations under resonant excitation and that the chirping velocity increases as we approach the critical excitation strength. The chirped amplitude mode enables us to determine the local modification of the effective potential even when the system is in a long-lived pre-thermal state. We then show that this chirped amplitude mode is an experimentally observable quantity since the photo-induced (super)-current in pump-probe experiments serves as an efficient proxy for the dynamics of the order parameter, including the chirped dynamics. Our result is based on the attractive Hubbard model using dynamical mean-field theory within the symmetry-broken state after a resonant excitation across the superconducting gap. Since the collective response takes place on emergently long timescales, we extend the hierarchical low-rank compression method for nonequilibrium Green's functions to symmetry-broken states and show that it serves as an efficient representation despite long-lived memory kernels.
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