Critical Solvation Structures Arrested Active Molecules for Reversible Zn Electrochemistry

Junjie Zheng,Bao Zhang, Xin Chen, Wenyu Hao,Jia Yao,Jingying Li,Yi Gan, Xiaofang Wang, Xingtai Liu,Ziang Wu, Youwei Liu,Lin Lv,Li Tao,Pei Liang,Xiao Ji,Hao Wang,Houzhao Wan

Nano-Micro Letters（2024）

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摘要

Highlights Critical solvation structure changes the hydrogen bond network through “catchers”. Catcher further arrests the active molecules to promote Zn 2+ deposition. The Zn||Zn symmetric battery can stably cycle for 2250 h. Zn||V 6 O 13 full battery achieved a capacity retention rate of 99.2% after 10,000 cycles.

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关键词

Zinc-ion battery,Critical solvation,Helmholtz layer,Arrest active molecule,Reversible zinc anode

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