Enhancing the performance of quasi-solid-state flexible supercapacitors with Ag and MnO2 co-decorated carbon nanofibrous electrodes
Electrochimica Acta(2024)
摘要
Flexible supercapacitors are gaining increasing popularity due to their potential in powering portable, wearable, and lightweight electronic devices. In this study, we have successfully developed a high-performance flexible electrode for quasi-solid-state supercapacitors by incorporating Ag into carbon nanofibers (CNF) through electrospinning, and growing MnO2 as an active material on the electrode using an in-situ redox method. The Ag and MnO2 co-decorated CNF electrode offers several advantages over conventional CNF electrodes, including an enlarged reaction area, higher charge storage capacity, and improved resistance to brittleness issues. Among all the quasi-solid-state supercapacitors tested, the MnO2-decorated electrode with an optimized Ag incorporation exhibited the highest specific capacitance of 184 F/g at a current density of 1 A/g, representing a remarkable 17-fold increase compared to the reference CNF electrode. Furthermore, the Ag and MnO2 co-decorated electrode demonstrated an energy density of 16.3 Wh/kg and a power density of 400 W/kg at the same current density. Notably, the electrode exhibited excellent flexibility, with a capacitance retention rate of 87 % when subjected to bending with a curvature ranging from 5 to 1.25 cm. Our results suggest that the Ag and MnO2 co-decorated CNF electrode holds great promise for flexible energy storage applications.
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关键词
Flexible supercapacitors,MnO2,Electrospinning,Carbon nanofibers
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