Features of phonon scattering by a spherical pore: Molecular dynamics insight

APPLIED PHYSICS LETTERS(2024)

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摘要
There is still a gap in understanding phonon scattering by geometrical defects at the nanoscale, and it remains a significant challenge for heat transfer management in nanoscale devices and systems. In this study, we aim to explore the characteristics of phonon scattering by a single pore to gain insights into thermal transport in nanostructures. The paper outlines a methodology for assessing the spatial distribution of the magnitude of the radial, azimuthal, and polar components of the velocity of scattered phonons by a spherical pore. We demonstrated that the size parameter, commonly employed in electromagnetic wave scattering theory, is vital in determining the scattering regime. Specifically, we show that the calculated scattering efficiency has the same pattern as that commonly obtained in classical wave scattering theory. However, we found that crystallographic directions are pivotal in shaping the scattering patterns, especially in the regions where scattering patterns are defined by the Mie resonances. This observation holds significance in understanding the influence of phonon coherence on thermal transport in nanostructured materials.
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