Flexible solid-state asymmetric supercapacitor based on reduced graphene oxide (rGO)/ruthenium oxide (RuO2) composite electrode
Journal of Alloys and Compounds(2024)
摘要
Energy storage in flexible supercapacitor devices extensively depends on electrode design with good electrochemical as well as mechanical properties. Here, a cost-effective and scalable method is proposed for the synthesis of a reduced graphene oxide/ruthenium oxide (rGO/RuO2) composite thin film for flexible supercapacitor. The successive ionic layer adsorption and reaction (SILAR) method used to synthesize rGO/RuO2 composite electrode allowed the synthesis of amorphous RuO2 with optimized rGO composition. The morphological structure of rGO/RuO2 composite examined using a scanning electron microscope showed compact spherical microparticles coated on rGO sheets. The electrochemical measurements of rGO/RuO2 composite electrode revealed that the composite material achieved a specific capacitance of 1371Fg-1 at a scan rate of 5mVs-1. Due to the combined impact of rGO and RuO2, a flexible solid-state asymmetric supercapacitor (FSS-ASC) of configuration rGO/RuO2/PVA-H2SO4/WO3 exhibited Cs of 114Fg-1 at 5mVs-1 with 88% of capacitance retention after 5,000 galvanostatic charge-discharge (GCD) cycles. The FSS-ASC provided a remarkable specific energy of 23Whkg-1 and a specific power of 613Wkg-1. The electrochemical features of rGO/RuO2 composite show a promising way to fabricate flexible supercapacitors.
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关键词
Asymmetric supercapacitor,Composite material, Reduced graphene oxide,Ruthenium oxide,Successive ionic layer adsorption and reaction (SILAR)
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