Large anomalous transverse transport properties in atomically thin 2D Fe 3 GaTe 2

Anomalous transverse conductivities, such as anomalous Hall conductivity (AHC), anomalous Nernst conductivity (ANC), and anomalous thermal Hall conductivity (ATHC), play a crucial role in the emerging field of spintronics. Motivated by the recent fabrication of two-dimensional (2D) ferromagnetic thin film Fe 3 GaTe 2 , we investigate the thickness-dependent anomalous transverse conductivities of the 2D Fe 3 GaTe 2 system (from one to four layers). The atomically ultrathin 2D Fe 3 GaTe 2 system shows above-room-temperature ferromagnetism with a large perpendicular magnetic anisotropy energy. Furthermore, we obtain a large AHC of −485 S/cm in the four-layer thickness, and this is further enhanced to −550 S/cm with small electron doping. This AHC is seven times larger than the measured AHC in thicker 2D Fe 3 GaTe 2 (178 nm). The ANC also reaches 0.55 A/K.m in the four-layer structure. Along with these, the four-layer system exhibits a large ATHC (−0.105 ~ −0.135 W/K.m). This ATHC is comparable to the large ATHC found in Weyl semimetal Co 3 Sn 2 S 2 . Based on our results, the atomically ultrathin 2D Fe 3 GaTe 2 system shows outstanding anomalous transverse conductivities and can be utilized as a potential platform for future spintronics and spin caloritronic device applications.