Predicting high-resolution air quality using machine learning: Integration of large eddy simulation and urban morphology data

Accurately predicting air pollutants, especially in urban areas with well-defined spatial structures, is crucial. Over the past decade, machine learning techniques have been widely used to forecast urban air quality. However, traditional machine learning approaches have limitations in accuracy and interpretability for predicting pollutants. In this study, we propose a convolutional neural network (CNN) model to predict the spatial distribution of CO concentration in Nanjing urban area at 10 m resolution. Our model incorporates various factors as input, such as building height, topography, emissions, and is trained against the outputs simulated by the parallelized large-eddy simulation model (PALM). The PALM model has 48 different scenarios that varied in emissions, wind speeds, and wind directions. The results display a strong consistency between the two models. Furthermore, we evaluate the performance of our model using a 10-fold cross-validation and out-of-sample cross-validation approach. This yields a robust correlation (with both R-2 > 0.8) and a low RMSE between the CO predicted by the PALM and CNN models, which demonstrates the generalization capability of our CNN model. The CNN can extract crucial features from the resulted weight contribution map. This map indicates that the CO concentration at a location is more influenced by nearby buildings and emissions than distant ones. The interpretable patterns uncovered by our model are related to neighborhood effects, wind speeds, directions, and the impact of orientation on urban CO distribution. The model also shows high prediction accuracy (R > 0.8) when applied to another city. Overall, the integration of our CNN framework with the PALM model enhances the accuracy of air quality predictions, while enabling a fluid dynamic laws interpretation, providing effective tools for air quality management.