Directing the persulfate activation reaction pathway by control of Fe-Nx/C single-atom catalyst coordination
Chemical Engineering Journal(2024)
摘要
•Single-atom Fe catalysts with different coordination numbers were simply prepared.•Fe-N3/C/PMS system exhibits excellent degradation performance of TC.•The coordination numbers of single-atom Fe regulates the activation pathway of PMS.•The free radical/non-free radical co-oxidation has high reactivity and stability.•Electron transfer mechanisms between Fe-Nx/C and PMS are proposed.
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关键词
Peroxymonosulfate,Single-atom Fe,Hybrid oxidation,Coordination structures,Electron transfer
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