Carrier confinement activated explicit solvent dynamic of CdS/BiVO4/H2O and optimized photocatalytic hydrogen evolution performances

Mingqi Yuan,Jagadeesh Suriyaprakash,Lianwei Shan,Huanyan Xu,Xuejiao Li,Haitao Wu,Guodao Ding,Ziqi Shi,Limin Dong,Feng_Ming Zhang

Journal of Colloid and Interface Science（2023）

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摘要

•Photogenerated electrons are entirely located in BiVO4 in CdS/BiVO4.•CdS substrate in CdS/BiVO4/H2O can enhance hydrogen diffusing rate.•Used solvation effect can provide rational ΔGH* in HER process.•O p orbital reforms the orbital energy level and activates the HER activity.

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关键词

CdS/BiVO4,Heterojunction,DFT,Hydrogen evolution reaction,Solvation

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