Magnetic Coupling between Fe(NO) Spin Probe Ligands Through Diamagnetic Ni ^II , Pd ^II and Pt ^II Tetrathiolate Bridges

Marcetta Y. Darensbourg,Manuel Quiroz,Molly M. Lockart, Shan Xue, D. Gareth Jones, Yisong Guo,Brad S. Pierce,Kim R. Dunbar,Michael B. Hall

Chemical Science（2023）

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摘要

The n d ( n = 3–5) orbital effects on the magnetic coupling within sulfur-bridged, iso-structural, tri-metallic complexes revealed that the heavier congeners significantly enhance superexchange between distal {Fe(NO)} 7 radicals: Pt ≫ Pd > Ni.

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spin probe ligands,<b>magnetic coupling,feno

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Magnetic Coupling between Fe(NO) Spin Probe Ligands Through Diamagnetic Ni II , Pd II and Pt II Tetrathiolate Bridges

Magnetic Coupling between Fe(NO) Spin Probe Ligands Through Diamagnetic Ni ^II , Pd ^II and Pt ^II Tetrathiolate Bridges