Strong magnetic exchange coupling in Ln₂ metallocenes attained by the trans-coordination of a tetrazinyl radical ligand

Niki Mavragani,Alexandros A. Kitos, J. Hrubý,Stephen Hill,Akseli Mansikkamäki,Jani O. Moilanen,Muralee Murugesu

Inorganic chemistry frontiers（2023）

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摘要

One of the strongest Ln-rad magnetic coupling was attained in a family of dinuclear Ln metallocenes via the trans coordination mode of a tetrazinyl-based radical bridge, with the Tb( iii ) and Dy( iii ) analogues exhibiting SMM behaviour.

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ln2 metallocenes,tetrazinyl radical ligand,strong magnetic exchange coupling,exchange coupling,trans-coordination

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Strong magnetic exchange coupling in Ln2 metallocenes attained by the trans-coordination of a tetrazinyl radical ligand

Strong magnetic exchange coupling in Ln₂ metallocenes attained by the trans-coordination of a tetrazinyl radical ligand