Cationic silyldiazenido complexes of the Fe(diphosphine)₂(N₂) platform: structural and electronic models for an elusive first intermediate in N₂ fixation

Adam D. Piascik, Peter J. Hill,Andrew D. Crawford,Laurence R. Doyle,Jennifer C. Green,Andrew E. Ashley

Chemical Communications（2017）

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摘要

Functionalisation of Fe-bound dinitrogen affords novel cationic silyldiazenido complexes, which are structural surrogates for unstable protonated intermediates in N2 fixation.

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Cationic silyldiazenido complexes of the Fe(diphosphine)2(N2) platform: structural and electronic models for an elusive first intermediate in N2 fixation

Cationic silyldiazenido complexes of the Fe(diphosphine)₂(N₂) platform: structural and electronic models for an elusive first intermediate in N₂ fixation