Initial reduction of CO₂ on perfect and O-defective CeO₂ (111) surfaces: towards CO or COOH?

Xiaoqing Lu,Weili Wang,Shuxian Wei,Chen Guo,Yang Shao,Mingmin Zhang,Zhigang Deng,Houyu Zhu,Wenyue Guo

RSC Advances（2015）

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摘要

CO₂ hydrogenation towards COOH is more favorable on perfect CeO₂ (111) surface, whereas reductive dissociation of CO₂ is predominant on O-defective surface. The O vacancy promotes reductive dissociation of CO₂ on O-defective CeO₂ (111) surface.

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cooh,initial reduction,surfaces,o-defective

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Initial reduction of CO2 on perfect and O-defective CeO2 (111) surfaces: towards CO or COOH?

Initial reduction of CO₂ on perfect and O-defective CeO₂ (111) surfaces: towards CO or COOH?