Avoiding dry reforming control in direct CH4 and CO2 conversion operating at low-temperature below ambient pressure over AgPd4-Fe3-δO4 nanocomposite

Elena Montejano-Nares,Blanca Martínez-Navarro, Eva Castillejos López,Esther Asedegbega-Nieto, Ángel Maroto Valiente, José M. Conesa Alonso,Inmaculada Rodríguez Ramos, Antonio R. Guerrero Ruíz,Francisco Ivars-Barceló

Chemical Engineering Journal（2023）

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摘要

•Direct conversion of methane and carbon dioxide not controlled by reforming reaction.•Oxygenated derivatives as main products by a purely heterogeneous catalysis process.•Cumulative productivities (acetone + dimethyl ether) reached above 260 mmol gcat-1h−1.•Dimethyl ether appears as secondary product formed via the acetone primary product.•Multiphasic nanocatalyst active and selective at low temperature bellow ambient pressure.

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关键词

Methane,Carbon dioxide,Heterogeneous catalysis,Mixed iron oxide,Acetone,Dimethyl ether

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