Magnetization process of cubic Fe3O4 submicron particles: First-order reversal curves and neutron diffraction studies

We have studied magnetization process of 260 nm sized cubic Fe3O4 particles below and above the Verwey transition temperature Tv similar to 110 K, by measurements of magnetic first-order reversal curves (FORCs) and high-resolution power neutron diffraction. The FORC diagram exhibits two distinct FORC distribution peaks below Tv, which shift towards the origin, merge into a single peak on heating, whereas only a single FORC peak appears above Tv. Neutron diffraction measurements under magnetic fields revealed a minimum of the magnetic intensity at a magnetic field of similar to-300 Oe, being close to the reversal field where the FORC peak is located. These results were interpreted as due to a reorientation and reversal of a spin vortex core, which accompany a large magnetic irreversibility.