Source Attribution of Atmospheric Dust Deposition to Utah Lake

HYDROLOGY(2023)

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摘要
Atmospheric deposition (AD) is a significant source of nutrient loading to waterbodies around the world. However, the sources and loading rates are poorly understood for major waterbodies and even less understood for local waterbodies. Utah Lake is a eutrophic lake located in central Utah, USA, and has high-nutrient levels. Recent research has identified AD as a significant source of nutrient loading to the lake, though contributions from dust particles make up 10% of total AD. To better understand the dust AD sources, we sampled suspected source locations and collected deposition samples around the lake. We analyzed these samples using Inductively Coupled Plasma (ICP) for 25 metals to characterize their elemental fingerprints. We then compared the lake samples to the source samples to determine likely source locations. We computed spectral angle, coefficient of determination, multi-dimensional scaling, and radar plots to characterize the similarity of the samples. We found that samples from local dust sources were more similar to dust in lake AD samples than samples from distant sources. This suggests that the major source of the dust portion of AD onto Utah Lake is the local empty fields south and west of the lake, and not the farther playa and desert sources as previously suggested. Preliminary data suggest that dust AD is associated with dry, windy conditions and is episodic in nature. We show that AD from dust particles is likely a small portion of the overall AD nutrient loading on Utah Lake, with the dry and precipitation sources contributing most of the load. This case identifies AD sources to Utah Lake and provides an example of data and methods that can be used to assess similarity or perform attribution for dust, soil, and other environmental data. While we use ICP metals, any number of features can be used with these methods if normalized.
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关键词
atmospheric deposition,nutrient loading,Utah Lake
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