Magnetic ground states in kagome YCu_3(OH)_6[(Cl_xBr_1-x)_3-y(OH)_y]

Aini Xu, Qinxin Shen,Bo Liu,Zhenyuan Zeng, Lankun Han,Liqin Yan, Jun Luo, Jie Yang, Rui Zhou,Shiliang Li

arxiv(2023)

引用 0|浏览6
暂无评分
摘要
Quantum spin liquids represent exotic states of spin systems characterized by long-range entanglement and emergent fractionalized quasiparticles. It is generally believed that disorder is hostile to quantum spin liquids. In our study, we investigated the magnetic properties of a kagome system, YCu_3(OH)_6[(Cl_xBr_1-x)_3-y(OH)_y]. Within this system, some of the hexagons exhibit alternate bonds along the Cu-O-Cu exchange paths, while others remain uniform. We found that a long-range antiferromagnetic order emerges when uniform hexagons dominate. Conversely, possible quantum-spin-liquid state arises when the number of alternate-bond hexagons exceeds about 2/3. Therefore, the alternate-bond hexagons, typically considered as disorders, actually serve as the building blocks of the quantum spin liquid in this system. Notably, the low-temperature properties of the quantum spin liquid are directly associated with the height of the out-of-plane yttrium ions, which may be linked to changes in superexchange energies. Our results suggest that understanding the magnetic ground states in this system lies beyond the theoretical framework of the Heisenberg model constructed on the kagome lattice.
更多
查看译文
AI 理解论文
溯源树
样例
生成溯源树,研究论文发展脉络
Chat Paper
正在生成论文摘要