A Co(TAML)-based artificial metalloenzyme for asymmetric radical-type oxygen atom transfer catalysis

Eva J. Meeus,Nico V. Igareta, Iori Morita,Thomas R. Ward,Bas de Bruin,Joost N. H. Reek

CHEMICAL COMMUNICATIONS（2023）

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摘要

We show that the incorporation of a biotinylated Co(TAML) cofactor within streptavidin enables asymmetric radical-type oxygen atom transfer catalysis with improved activity and enantioselectivity. We show that the incorporation of a biotinylated Co(TAML) cofactor within streptavidin enables asymmetric radical-type oxygen atom transfer catalysis with improved activity and enantioselectivity.

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