Bifunctional CoFe/HZSM-5 catalysts orient CO2 hydrogenation towards liquid hydrocarbons

Kai Wang,Na Liu,Jian Wei,Yang Yu,Jixin Zhang,Joshua Iseoluwa Orege, Lifei Song,Qingjie Ge,Jian Sun

Chemical communications (Cambridge, England)（2023）

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摘要

Converting CO2 to liquid (C5+) hydrocarbons remains a significant hurdle. Our study shows that CoFe/HZSM-5 boosts C5+ selectivity to 73.4%, up from 59% for Fe/HZSM-5. This study highlights the pivotal roles of zeolite acidity and catalyst proximity in this improvement. These insights pave the way for more effective CO2 utilization.

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