Copper oxide in layered tin oxide with intracrystalline microporosity for oxidative imination of toluene and p-xylene

Gautam Gogoi, Nand K. Gaur,Seonghwan Lee,Young-Bin Park,Lakshi Saikia,Magdi E.A. Zaki,Kusum K. Bania

Molecular Catalysis（2023）

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摘要

•CuO loaded in layered SnO2 with crystalline microporosity.•CuO-SnO2 appeared as excellent non-noble metal catalyst for oxidative imination of toluene and p-xylene.•Intracrystalline microporosity favored the diffusion-controlled reaction.•Cation-pi interaction played a dominant role in selective transformation.•The mechanistic understanding through DFT studied.

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关键词

Toluene,Xylene,Copper oxide in layered tin oxide (SnO2),Imine,DFT-calculation,Mechanism

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