Amine-modified polyionic liquid supports enhance the efficacy of PdNPs for the catalytic hydrogenation of CO₂ to formate

Reece Paterson, Luke E. Fahy,Elisabetta Arca,Casey Dixon,Corinne Y. Wills, Han Yan,Anthony Griffiths,Sean M. Collins,Kejun Wu,Richard A. Bourne,Thomas W. Chamberlain,Julian G. Knight,Simon Doherty

Chemical communications (Cambridge, England)（2023）

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摘要

Palladium nanoparticles stabilised by aniline modified polymer immobilised ionic liquid is a remarkably active catalyst for the hydrogenation of CO2 to formate; the initial TOF of 500 h(-1) is markedly higher than either unmodified catalyst or its benzylamine and N,N-dimethylaniline modified counterparts and is among the highest to be reported for a PdNP-based catalyst.

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catalytic hydrogenation,co2,amine-modified

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Amine-modified polyionic liquid supports enhance the efficacy of PdNPs for the catalytic hydrogenation of CO2 to formate

Amine-modified polyionic liquid supports enhance the efficacy of PdNPs for the catalytic hydrogenation of CO₂ to formate