Unraveling the thallium immobilization in CuO/PMS system

Zhujun Liu,Xinning Dai, Jun He,Wei Chen,Yuxin Wei, Qiaoling Zhou,Dandan Ma,Xinyu Zheng

Chemical Engineering Journal（2023）

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摘要

•CuO/PMS system was first established for the immobilization of dissolved Tl(I).•1O2 and OH facilitated Tl(I) to Tl(III) conversion.•Electrostatic attraction and surface precipitation enhanced Tl immobilization.•Tl(H2O)33+ hydrate stably adsorbed onto CuO (111) surface than Tl(H2O)2+ hydrate.

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关键词

Thallium, CuO nanoparticles, Catalysis, Adsorption, Theoretical calculations

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