Zr-MOF catalyzed selective oxidation of anilines to azoxybenzenes in aqueous H2O2 solution

Jianhong Zheng,Xi Chen, Xiaoxiao Yin,Kai Chen,Aili Liu,Xiaochun Yu,Shun Wang,Zhongwei Chen

MOLECULAR CATALYSIS（2023）

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摘要

•A highly efficient Zr-MOF/H2O2 catalytic system was developed for selective aniline oxidation.•The impact of metal, organic linker, and pore size on catalytic performance was studied.•Quantitative yield of azoxybenzene and high H2O2 efficiency was achieved.•The H2O2 activation mechanism based on bridging Zr-OH-Zr sites was proposed.

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关键词

MOF,Selective aniline oxidation,H2O2,Organic solvent-free

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