Dissolution of (U,Th)O2 heterogeneous mixed oxides

C. Hours,L. Claparede, N. Reynier-Tronche, I. Viallard,R. Podor,N. Dacheux

JOURNAL OF NUCLEAR MATERIALS(2023)

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摘要
•Polished heterogeneous U1-xThxO2 pellets have been prepared, characterized then submitted to dissolution tests in nitric acid solutions.•Different behaviours during dissolution have been observed between embedding U-enriched phase and Th-enriched heterogeneities.•Increasing the quantity of heterogeneities in the pellets led to the decrease of the dissolution rates.•U1-xThxO2 sintered powders with x > 0.58 dissolved slowly in the absence of HNO2 catalytic species.
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关键词
Nuclear fuel,Heterogeneous pellets,Mixed oxide,Dissolution
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