Effect of water on CO2 absorption by a novel anhydrous biphasic absorbent: Phase change behavior, absorption performance, reaction heat, and absorption mechanism

Wufeng Jiang,Xiaoyi Gao, Bin Xu,Ge Gao,Fan Wu,Xiaoshan Li,Liqi Zhang,Cong Luo

Separation and Purification Technology（2023）

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摘要

•Water markedly affected phase change behaviors of anhydrous biphasic absorbents.•The presence of water was negative for CO2 absorption but beneficial to desorption.•The main CO2-product was HCO3- in the presence of water rather than carbamate.•Effect of water on CO2 absorption mechanism of [N1111][Gly]/ethanol was clarified.

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关键词

Water effects,Biphasic absorbent,Glycinate ionic liquids,Reaction mechanism,Carbon dioxide capture

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