Nitrogen amended graphene catalyses fast reduction of vinyl chloride by nano zerovalent iron

Qiong Ouyang,Hans Christian Bruun Hansen,Lisbeth Garbrecht Thygesen,Dominique J. Tobler

Water research（2023）

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摘要

•Nitrogen-doped graphene (NG) enables fast vinyl chloride (VC) reduction by nZVI.•Co-pyrolysis of urea and graphene at 950 °C yielded NG with highest reactivity.•NG reactivity correlates with density of pyridine-N-oxide and structural defects.•NG reactivity is attributed to atomic hydrogen storage and electron mediation.

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关键词

Dechlorination,Carbonaceous materials,Chlorinated ethylenes,Electron transfer,Hydrogen spill-over

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