Realizing fast Li-ion conduction of Li₃PO₄ solid electrolyte at low temperature by mechanochemical formation of lithium-containing dual-shells

Shunqin Zeng,Xiaoli Ding,Liqing He,Hai-Wen Li,Qingan Zhang,Yongtao Li

MATERIALS ADVANCES（2023）

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摘要

Dual lithium-containing hydride/oxide shells are constructed by in situ mechano-induced assembly of Li3PO4 reacting with LiBH4. The ionic conductivity of the Li3PO4-based composite is promoted nearly 4 orders of magnitude, up to 0.04 mS cm(-2) at 75 & DEG;C as compared to the pure one, possessing an electrochemical window of -0.2-5 V (vs. Li/Li+).

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solid electrolyte,li-ion,lithium-containing,dual-shells

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Realizing fast Li-ion conduction of Li3PO4 solid electrolyte at low temperature by mechanochemical formation of lithium-containing dual-shells

Realizing fast Li-ion conduction of Li₃PO₄ solid electrolyte at low temperature by mechanochemical formation of lithium-containing dual-shells