The formation of high CO2 loading solid phase from 1,4-butanediamine/ethylene glycol biphasic solvent: Phase-changing behavior and mechanism

Cunshi Wang,Gongkui Xiao,Xiaobin Zhou,Qiuzi Zhu,Yuanyi Chen,Zhimin Gao,Chao Liu,Jianzhong Zhu

Separation and Purification Technology（2023）

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摘要

•A novel biphasic solvent with a high CO2 loading in the solid phase was developed for CCUS.•The formation of H-bonding between EG and BDA was confirmed.•Particle self-aggregation induces the liquid–solid phase transition.•The interaction between the absorbed products was elucidated by ESP and IGMH analysis.•The phase-change mechanism of CO2 absorption into BDA/EG system was elucidated.

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关键词

CO2 absorption,Non-aqueous,Liquid-solid phase change,Alkyl-carbonate,Mechanism

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